A study of the ferromagnetic transition of SrRuO3 in nanometer thick bilayers with YBa2Cu3Oy, La1.88Sr0.12CuO4-y, Au and Cr: Signature of injected carriers in the pseudogap regime

Abstract

The hypothesis regarding the existence of uncorrelated pre-formed pairs in the pseudogap regime of superconducting YBa2Cu3Oy is tested experimentally using bilayers of YBa2Cu3Oy and the itinerant ferromagnet SrRuO3. In our study, we monitor the influence of YBa2Cu3Oy on Tp, the ferromagnetic ordering temperature of SrRuO3. Here, Tp is the temperature of maximum dM/dT or dR/dT where M and R are the magnetization and resistance of SrRuO3, respectively. We compare the results with similar measurements carried out on bilayers of La1.88Sr0.12CuO4-y, Au and Cr with SrRuO3. We find that in bilayers made of underdoped 10 nm YBa2Cu3Oy/5 nm SrRuO3, the Tp values are shifted to lower temperatures by up to 6-8 K as compared to Tp≈ 140 K of the 5 nm thick reference SrRuO3 film. In contrast, in the other type of bilayers, which are not in the pseudogap regime near Tp, only a smaller shift of up to 2 K is observed. These differences are discussed in terms of a proximity effect, where carriers from the YBa2Cu3Oy layer are injected into the SrRuO3 layer and vice versa. We suggest that correlated electrons in the pseudogap regime of YBa2Cu3Oy are responsible for the observed large Tp shifts.

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