Magneto-elastic coupling in hexagonal YMnO3
Abstract
We report an ultrasonic investigation of the elastic moduli on a single crystal of hexagonal YMnO3 as a function of temperature. Stiffening anomalies in the antiferromagnetic N\'eel state below TN = 72.4 K are observed on all the four elastic moduli Cii. The anomalies are the most important on C11 and C66 for in-plane elastic deformations; this is consistent with a strong coupling of the lattice with the in-plane exchange interactions. We use a Landau free energy model to account for these elastic anomalies. We derive an expression which relates the temperature profile of the anomaly to the order parameter; the critical exponent associated to this parameter β = 0.42 is not consistent with a chiral XY or 3D Heisenberg universality class, but more in agreement with a conventional antiferromagnetic long range order. A tiny softening anomaly on C11 for which hysteresis effects are observed could be indicative of an interaction between ferroelectric and magnetic domains at TN. Moreover, magnetic fluctuations effects both above and below TN are identified through abnormal temperature and magnetic field effects.
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