Shaping single walled nanotubes

Abstract

We show that electron irradiation in a dedicated scanning transmission microscope can be used as a nano-electron-lithography technique allowing the controlled reshaping of single walled carbon and boron nitride nanotubes. The required irradiation conditions have been optimised on the basis of total knock-on cross sections calculated within density functional based methods. It is then possible to induce morphological modifications, such as a change of the tube chirality, by removing severals tens of atoms with a nanometrical spatial resolution. These irradiation techniques could open new opportunities for nano-engeneering a large variety of nanostructured materials.