Observation of magnetization reversal and negative magnetization in a double perovskite compound Sr2YbRuO6

Abstract

Detailed magnetic properties of the compound Sr2YbRuO6 are presented here. The compound belongs to the family of double perovskites forming a monoclinic structure. Magnetization meas-urements reveal clear evidence for two components of magnetic ordering aligned opposite to each other, leading to a magnetization reversal, compensation temperature (T* = 34 K) and neg-ative magnetization at low temperatures and low magnetic fields. Heat capacity measurements corroborate the presence of two components in the magnetic ordering and a noticeable third anomaly at low temperatures (~15 K) which cannot be attributed the Schottky effect. The calcu-lated magnetic entropy is substantially lower than that expected for the ground states of the or-dered moments of Ru5+ and Yb3+, indicating the presence of large crystal field effects and/ or in-complete magnetic ordering and/or magnetic frustrations well above the magnetic ordering. An attempt is made to explain the magnetization reversal within the frameworks of available models.