Electronic and structural transition in La0.2 Sr0.8 Mn O3

Abstract

We investigate the interplay of the electronic and structural transition in La0.2Sr0.8MnO3. The transport and specific heat measurements exhibit unusual evolutions and signature of a first order phase transition around 265 K. Mn K-edge extended x-ray absorption fine structure results reveal distortion in the MnO6 octahedra even in the cubic phase and a remarkable evolution of the distortion across the phase transition. These results manifest the importance of fluctuations in Mn 3d orbital occupancy and disorder in their electronic properties, which may help in understanding the orbital and spin ordering proposed in these systems.

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