Different resistivity response to spin density wave and superconductivity at 20 K in Ca1-xNaxFe2As2

Abstract

We report that intrinsic transport and magnetic properties, and their anisotropy from high quality single crystal CaFe2As2. The resistivity anisotropy (c/ab) is 50 , and less than 150 of BaFe2As2, which arises from the strong coupling along c-axis due to an apparent contraction of about 0.13 nm compared to BaFe2As2. Temperature independent anisotropy indicates that the transport in ab plane and along c-axis direction shares the same scattering mechanism. In sharp contrast to the case of parent compounds ROFeAs (R=rare earth) and MFe2As2 (M=Ba and Sr), spin-density-wave (SDW) ordering (or structural transition) leads to a steep increase of resistivity in CaFe2As2. Such different resistivity response to SDW ordering is helpful to understand the role played by SDW ordering in Fe-based high-Tc superconductors. The susceptibility behavior is very similar to that observed in single crystal BaFe2As2. A linear temperature dependent susceptibility occurs above SDW transition of about 165 K. Partial substitution of Na for Ca suppresses the SWD ordering (anomaly in resistivity) and induces occurrence of superconductivity at 20 K.

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