Distinct pseudogap and superconducting state quasiparticle relaxation dynamics in near-optimally doped SmFeAsO0.8F0.2 single crystals

Abstract

We use femtosecond spectroscopy to investigate the quasiparticle relaxation and low-energy electronic structure in a near-optimally doped pnictide superconductor with Tc=49.5 K. Multiple relaxation processes are evident, with distinct superconducting state quasiparticle (QP) recombination dynamics exhibiting a T-dependent superconducting (SC) gap, and a clear "pseudogap" (PG) -like feature with an onset around 200K indicating the existence of a temperature-independent gap of magnitude PG= 61 +- 9 meV above Tc. Both the SC and PG components show saturation as a function of fluence with distinct saturation thresholds ~0.15 μJ/cm2 and 1.5 μJ/cm2, respectively.

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