Towards the theory of ferrimagnetism II

Abstract

The present paper is a sequel to the paper by Karchev (2008 J.Phys.:Condens.Matter 20 325219). A two-sublattice ferrimagnet, with spin-s1 operators S1i at the sublattice A site and spin-s2 operators S2i at the sublattice B site, is considered. Renormalized spin-wave theory, which accounts for the magnon-magnon interaction, and its extension are developed to describe the two ferrimagnetic phases (0,T*) and (T*,TN) in the system, and to calculate the magnetization as a function of temperature. The influence of the parameters in the theory on the characteristic temperatures TN and T* is studied. It is shown that, increasing the inter-sublattice exchange interaction, the ratio TN/T*>1 decreases approaching one, and above some critical value of the exchange constant there is only one phase TN = T*, and the magnetization-temperature curve has the typical Curie-Weiss profile. When the intra-exchange constant of sublattice with stronger intra-exchange interaction increases the Neel temperature increases while T* remains unchanged. Finally, when the magnetic order of the sublattice with smaller magnetic order decreases, T* decreases. The theoretical predictions are utilize to interpret the experimentally measured magnetization-temperature curves.

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