Gigantic magnetoelectric effect caused by magnetic-field-induced canted antiferromagnetic-paramagnetic transition in quasi-two-dimensional Ca$_2$CoSi$_2$O$_7$ crystal

Abstract

We have investigated the magnetic and dielectric properties of Ca$_2$CoSi$_2$O$_7$ crystal. The dielectricity and magnetism of Ca$_2$CoSi$_2$O$_7$ are strongly coupled below a canted antiferromagnetic transition temperature ($T_{\rm N}$): Magnetic fields induce electric polarization below $T_{\rm N}$. Interestingly, the magnetic-field-induced electric polarization is detected even without poling electric fields. Below $T_{\rm N}$, a canted antiferromagnetic-paramagnetic transition is induced by magnetic fields. The large magnetocapacitance is observed around $T_{\rm N}$. The origin of the large magnetocapacitance is due to the magnetic-field-induced the canted antiferromagnetic-paramagnetic transition.