Phase diagram of CeFeAs1-xPxO obtained from electric resistivity, magnetization, and specific heat measurements

Abstract

We performed a systematic study on the properties of CeFeAs1-xPxO (0≤ x≤ 1) by electrical resistivity, magnetization and specific heat measurements. The c-axis lattice constant decreases significantly with increasing P content, suggesting a remarkable chemical pressure. The Fe-3d electrons show the enhanced metallic behavior upon P-doping and undergo a magnetic quantum phase transition around x ≈ 0.4. Meanwhile, the Ce-4f electrons develop a ferromagnetic order near the same doping level. The ferromagnetic order is vanishingly small around x=0.9. The data suggest a heavy-fermion-like behavior as x≥ 0.95. No superconductivity is observed down to 2 K. Our results show the ferromagnetic ordered state as an intermediate phase intruding between the antiferromagnetic bad metal and the nonmagnetic heavy fermion metal and support the cerium-containing iron pnictides as a unique layered Kondo lattice system.

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