Interplay between the Kondo effect and randomness: Griffiths phase in MxTiSe2 (M = Co, Ni, and Fe) single crystals

Abstract

We investigate the interplay between the Kondo effect and randomness in MxTiSe2 (M = Co, Ni, and Fe) single crystals. Although the typical low-T upturn of resistivity implies the Kondo effect around the single-ion Kondo temperature TK, positive magnetoresistance linearly proportional to the magnetic field and the power-law scaling of magnetization suggest the forbidden coexistence between Kondo effect and time reversal symmetry breaking. This puzzling result is resolved by the Griffiths scenario - disorder-induced distribution of the Kondo temperature produces an effective Kondo temperature (TK) much lower than TK, allowing unscreened local moments above TK and resulting in non-Fermi liquid properties in MxTiSe2 below the percolation threshold (x<xc).

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