Upper critical field and thermally activated flux flow in single crystalline Tl0.58Rb0.42Fe1.72Se2

Abstract

The upper critical field μ0Hc2(Tc) of Tl0.58Rb0.42Fe1.72Se2 single crystals has been determined by means of measuring the electrical resistivity in both a pulsed magnetic field (60T) and a DC magnetic field (14T). It is found that Hc2 linearly increases with decreasing temperature for H, reaching μ0Hc2H c(0K)60 T. On the other hand, a larger μ0Hc2(0K) with a strong convex curvature is observed for H (μ0Hc2H c(18K)60T). This compound shows a moderate anisotropy of the upper critical field around Tc, but decreases with decreasing temperature. Analysis of the upper critical field based on the Werthamer-Helfand-Hohenberg (WHH) method indicates that μ0Hc2(0K) is orbitally limited for H, but the effect of spin paramagnetism may play an important role on the pair breaking for H. All these experimental observations remarkably resemble those of the iron pnictide superconductors, suggesting a unified scenario for the iron-based superconductors. Moreover, the superconducting transition is significantly broadened upon applying a magnetic field, indicating strong thermal fluctuation effects in the superconducting state of Tl0.58Rb0.42Fe1.72Se2. The derived thermal activation energy for vortex motion is compatible with those of the 1111-type iron pnictides.

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