Unusual Field-Insensitive Phase Transition and Kondo Behavior in SmTi2Al20
Abstract
Magnetization, electrical resistivity and specific heat measurements were performed on high-quality single crystalline SmTi2Al20 (residual resistivity ratio 40) grown by Al self-flux method. A Kondo-like T dependence in the resistivity is observed below 50 K. We discovered a field-insensitive phase transition at Tx = 6.5 K and a field-insensitive heavy fermion behavior with the electronic specific heat coefficient γ = 150 mJ/(K2 mol). Specific heat analysis reveals that the ground state is a 8 quartet state and the Sm magnetic dipole moment m Sm ( 0.5 μ B at T 0) orders below Tx in spite of the field-insensitive behavior. Possible reasons for the field insensitiveness will be discussed.
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