Microscopic coexistence of antiferromagnetic order and superconductivity in Ba0.77K0.23Fe2As2

Abstract

We report 75As nuclear magnetic resonance studies on an underdoped single-crystal Ba0.77K0.23Fe2As2 with Tc = 16.5 K. Below TN = 46 K, the NMR peaks for H//c split and those for H //a shift to higher frequencies, which indicates that an internal magnetic field along the c axis develops below TN. The spin-lattice relaxation rate 1/T1 measured at the shifted peak with H//a, which experiences the internal field, shows a distinct decrease below Tc(μ0H = 12 T) = 16 K, following a T3 relation at low temperatures. Our results show unambiguously that antiferromagnetic order and superconductivity coexist microscopically. The unusual superconducting state with the coexisting magnetism is highlighted.

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