Coherent phase control in ionization of Magnesium by a bichromatic laser field of frequencies ω and 2ω

Abstract

We have investigated the coherent phase control on the (3p2) autoionizing state (AIS) resonantly coupled with the ground state for Mg through a two- and a four-photon transition simultaneously, using a bichromatic linearly polarized laser field. The frequency is chosen such that the lasers are tunable around resonance with the transition (3s2(1Se)→ 3p2(1Se)), which implies (ωf=2.11) eV and (ωh=4.22) eV. We are interested in the modification of autoionizing (AI) line shape through the relative phase and laser intensities. A strong phase dependence on the total ionization yield and ionization rate is found. We also performed a time-dependent calculation which takes into consideration all the resonant states of the process.

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