Optically induced currents in dielectrics as a nonlinear optical effect

Abstract

We show that recently observed DC currents produced by below-the-bandgap femtosecond pulses [1] can be explained as nonlinear optical effects based on multi-photon quantum interference and creation of an asymmetric distribution of virtual carriers in the conduction and valence bands. We establish an unambiguous connection between the nonlinear optical conductivity responsible for the observed DC currents and charges and the odd-order nonlinear optical susceptibilities of the material. Using a single well known measured value of the third order susceptibility (nonlinear index) of SiO2 we obtain excellent agreement with all the experimental data of [1] without resorting to extensive numerical modeling. A clear physical picture of the origin of the photo-induced currents and charges shows that the versatility of ultrafast (virtual) nonlinear optical phenomena extends even further than had been previously thought.