Self-organized pattern formation in laser-induced multiphoton ionization

Abstract

We use finite-difference time-domain modelling to investigate plasma generation induced by multi-photon absorption of intense laser light in dielectrics with tiny inhomogenities. Plasma generation is found to be strongly amplified around nanometer-sized inhomogeneities as present in glasses. Each inhomogeneity acts as the seed of a plasma structure growing against the direction of light propagation. Plasma structures originating from randomly distributed inhomogeneities are found to interact strongly and to organize in regularly spaced planes oriented perpendicularly to the laser polarization. We discuss similarities between our results and nanogratings in fused silica written by laser beams with spatially homogeneous as well as radial and azimuthal polarization.