Slow Exciton Spin Relaxation in Single Self-Assembled In$_{1-x}$Ga$_x$As/GaAs Quantum Dots

Abstract

We calculate the acoustic phonon-assisted exciton spin relaxation in single self-assembled In$_{1-x}$Ga$_x$As/GaAs quantum dots using an atomic empirical pseudopotential method. We show that the transition from bright to dark exciton states is induced by Coulomb correlation effects. The exciton spin relaxation time obtained from sophisticated configuration interaction calculations is approximately 15--55 $\mu$s in pure InAs/GaAs QDs and even longer in alloy dots. These results contradict previous theoretical and experimental results, which suggest very short exciton spin times (a few ns), but agree with more recent experiments that suggest that excitons have long spin relaxation times ($>$ 1 $\mu$s).