Temperature dependence of electronic and magnetic properties of (DOEO)4[HgBr4]TCE single crystals
Abstract
The temperature dependence of electronic and magnetic properties of the organic charge-transfer salt (DOEO)4[HgBr4]TCE was investigated using magnetometry. Electronic transport properties revealed three distinct phases which are related to different magnetic coupling phenomena. In the low-temperature insulating phase (T<70 K) the antiferromagnetic coupling between two distinct sites of magnetic moments causes antiferromagnetic order below the N\'eel temperature TN=40 K. In the temperature region 70-120 K the (DOEO)4[HgBr4]TCE shows metallic-like behavior and with further increasing of temperature it becomes a bad metal due to loss of itinerant character and increase of hopping conductivity of charge carriers.
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