Fano Interference at the Excitation of Coherent Phonons: Relation between the Asymmetry Parameter and the Initial Phase of Coherent Oscillations

Abstract

The theoretical assertion that the Fano asymmetry parameter and the asymptotic initial phase of a harmonic oscillator interacting with a continuum are interrelated is experimentally verified. By an example of coherent fully symmetric A1g phonons in bismuth that are excited by ultrashort laser pulses at liquid helium temperature, it is demonstrated that, for negative values of the asymmetry parameter, the asymptotic phase increases as the modulus of the parameter decreases.