Spin-flop transition and magnetic phase diagram in CaCo2As2 revealed by torque measurements

Abstract

The magnetic properties of CaCo2As2 single crystal was systematically studied by using dc magnetization and magnetic torque measurements. A paramagnetic to antiferromagnetic transition occurs at TN = 74 K with Co spins being aligned parallel to the c axis. For H c, a field-induced spin-flop transition was observed below TN and a magnetic transition from antiferromagnetic to paramagnetic was inferred from the detailed analysis of magnetization and magnetic torque. Finally, we summarize the magnetic phase diagram of CaCo2As2 based on our results in the H-T plane.

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