Strong Cavity-Pseudospin Coupling in Monolayer Transition Metal Dichalcogenides: Spontaneous Spin-Oscillations and Magnetometry

Abstract

Strong coupling between the electronic states of monolayer transition metal dichalcogenides (TMDC) such as MoS2, MoSe2, WS2, or WSe2, and a two-dimensional (2D) photonic cavity gives rise to several exotic effects. The Dirac type Hamiltonian for a 2D gapped semiconductor with large spin-orbit coupling facilitates pure Jaynes-Cummings type coupling in the presence of a single mode electric field. The presence of an additional circularly polarized beam of light gives rise to valley and spin dependent cavity-QED properties. The cavity causes the TMDC monolayer to act as an on-chip coherent light source and a spontaneous spin-oscillator. In addition, a TMDC monolayer in a cavity is a sensitive magnetic field sensor for an in-plane magnetic field.

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