Polaron master equation theory of pulse driven phonon-assisted population inversion and single photon emission from quantum dot excitons

Abstract

We introduce an intuitive and semi-analytical polaron master equation approach to model pulse-driven population inversion and emitted single photons from a quantum dot exciton. The master equation theory allows one to identify important phonon-induced scattering rates analytically, and fully includes the role of the time-dependent pump field. As an application of the theory, we first study a quantum dot driven by a time-varying laser pulse on and off resonance, showing the population inversion caused by acoustic phonon emission in direct agreement with recent experiment of Quilter {\em et al.}, Phys Rev Lett {\bf 114}, 137401 (2015). We then model quantum dots in weakly coupled cavities and show the difference in population response between exciton-driven and cavity-driven systems. Finally, we assess the nonresonant phonon-assisted loading scheme with a quantum dot resonantly coupled to a cavity as a deterministic single photon source, and compare and contrast the important figures of merit with direct Rabi oscillation of the population using a resonant $\pi$ pulse, where the latter is shown to be much more efficient.