Band structure reconstruction across nematic order in high quality FeSe single crystal as revealed by optical spectroscopy study

Abstract

We perform an in-plane optical spectroscopy measurement on high quality FeSe single crystals grown by a vapor transport technique. Below the structural transition at $T_{\rm s}\sim$90 K, the reflectivity spectrum clearly shows a gradual suppression around 400 cm$^{-1}$ and the conductivity spectrum shows a peak at higher frequency. The energy scale of this gap-like feature is comparable to the width of the band splitting observed by ARPES. The low-frequency conductivity consists of two Drude components and the overall plasma frequency is smaller than that of the FeAs based compounds, suggesting a lower carrier density or stronger correlation effect. The plasma frequency becomes even smaller below $T_{\rm s}$ which agrees with the very small Fermi energy estimated by other experiments. Similar to iron pnictides, a clear temperature-induced spectral weight transfer is observed for FeSe, being indicative of strong correlation effect.