Unique magnetic structure of YbCo2Si2

Abstract

We report on the results of powder and single crystal neutron diffraction to investigate the magnetic order in YbCo2Si2 below the N\'eel temperature T N = 1.7~K in detail. Two different magnetically ordered phases can clearly be distinguished. At lowest temperatures a commensurate magnetic structure with a propagation vector k1 = (0.25~ 0.25~ 1) is found, while the intermediate phase (T > 0.9~K) is characterized by an incommensurate magnetic structure with k2 = (0.25~ 0.086~ 1). The magnetic structure in YbCo2Si2 is in marked contrast to all other known RCo2Si2 compounds (R = rare earth element) likely due to some itineracy of the Yb 4f states being responsible for the magnetism.

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