Nature of the Antiferromagnetic and Nematic Transitions in Sr$_{1-x}$Ba$_x$Fe$_{1.97}$Ni$_{0.03}$As$_2$

Abstract

We have systematically studied the antiferromagnetic and nematic transitions in Sr$_{1-x}$Ba$_x$Fe$_{1.97}$Ni$_{0.03}$As$_2$ by magnetic susceptibility and uniaxial-pressure resistivity measurements, respectively. The derivatives of the temperature dependence of both magnetic and nematic susceptibilities show clearly sharp peak when the transitions are first-order. Accordingly, we show that while both of the magnetic and nematic transitions change from first-order to second-order with increasing Barium doping level, there is a narrow doping range where the former becomes second-order but the latter remains first-order, which has never been realized before in other systems. Moreover, the antiferromagnetic and nematic transition temperatures become different and the jump of nematic susceptibility becomes small in this intermediate doping range. Our results provide key information on the interplay between magnetic and nematic transitions. Concerning the current debate on the microscopic models for nematicity in iron-based superconductors, these observations agree with the magnetic scenario for an itinerant fermionic model in excellent details.