Quasicontinuum γ-decay of 91,92Zr: benchmarking indirect (n,γ) cross section measurements for the s-process

Abstract

Nuclear level densities (NLDs) and γ-ray strength functions (γSFs) have been extracted from particle-γ coincidences of the 92Zr(p,p' γ)92Zr and 92Zr(p,d γ)91Zr reactions using the Oslo method. The new 91,92Zr γSF data, combined with photonuclear cross sections, cover the whole energy range from Eγ ≈ 1.5~MeV up to the giant dipole resonance at Eγ ≈ 17~MeV. The wide-range γSF data display structures at Eγ ≈ 9.5~MeV, compatible with a superposition of the spin-flip M1 resonance and a pygmy E1 resonance. Furthermore, the γSF shows a minimum at Eγ ≈ 2-3~MeV and an increase at lower γ-ray energies. The experimentally constrained NLDs and γSFs are shown to reproduce known (n, γ) and Maxwellian-averaged cross sections for 91,92Zr using the TALYS reaction code, thus serving as a benchmark for this indirect method of estimating (n, γ) cross sections for Zr isotopes.

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