Magnetotransport properties of MoP2

Abstract

We report magnetotransport and de Haas-van Alphen (dHvA) effect studies on MoP2 single crystals, predicted to be type-2 Weyl semimetal with four pairs of robust Weyl points located below the Fermi level and long Fermi arcs. The temperature dependence of resistivity shows a peak before saturation, which does not move with magnetic field. Large nonsaturating magnetoresistance (MR) was observed, and the field dependence of MR exhibits a crossover from semicalssical weak-field B2 dependence to the high-field linear-field dependence, indicating the presence of Dirac linear energy dispersion. In addition, systematic violation of Kohler's rule was observed, consistent with multiband electronic transport. Strong spin-orbit coupling (SOC) splitting has an effect on dHvA measurements whereas the angular-dependent dHvA orbit frequencies agree well with the calculated Fermi surface. The cyclotron effective mass 1.6me indicates the bands might be trivial, possibly since the Weyl points are located below the Fermi level. Interestingly, quasi-two dimensional(2D) band structure is observed even though the crystal structure of MoP2 is not layered.

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