Tailored Raman-resonant four-wave-mixing process

Abstract

Nonlinear optical processes are strongly dominated by phase relationships among electromagnetic fields that are relevant to its optical process. In this paper, we theoretically and experimentally show, as a typical example, that in a Raman-resonant four-wave-mixing process, the first anti-Stokes and Stokes generations can be tailored to a variety of forms by manipulating the phase relationships among the relevant electromagnetic fields.