Magnetic State Selected by Magnetic Dipole Interaction in Kagome Antiferromagnet NaBa2Mn3F11
Abstract
We have studied the ground state of the classical Kagome antiferromagnet NaBa2Mn3F11. Strong magnetic Bragg peaks observed in the d-spacing shorter than 6.0 \ were indexed by the propagation vectors of k0 = (0,0,0). Additional peaks with weak intensities in the range of the d-spacing longer than 8.0 \ were indexed by the incommensurate vectors of k1=(0.3209(2),0.3209(2),0) and k2=(0.3338(4),0.3338(4),0). Magnetic structure analysis exhibits that the 120 structure with the tail-chase geometry having k0 is modulated by the incommensurate vectors. The classical calculation of the Kagome Heisenberg antiferromagnet having the antiferromagnetic 2nd-neighbor interaction, the ground state of which is degenerated 120 structures with k0, reveals that the magnetic dipole-dipole (MDD) interaction including up to the 4th neighbor terms selects the tail-chase structure. The observed modulation of the tail-chase structure is indicated to be due to a small perturbation such as the long-range MDD interaction or the interlayer interaction.
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