Theory of Orbital Magnetic Quadrupole Moment and Nonlinear Anomalous Thermoelectric Transport

Abstract

We present a microscopic theory of the magnetic quadrupole moment density $\mathcal{Q}_{ij}$ in periodic crystals with combined time reversal ($\mathcal{T}$) and inversion ($\mathcal{I}$) symmetry. We obtain a gauge-invariant expression with clear physical interpretation and demonstrate the typical behaviour of $\mathcal{Q}_{ij}$ in a minimal two-band model that hosts a tilted Dirac cone. We then show that $\mathcal{Q}_{ij}$ leads to an intrinsic nonlinear anomalous thermoelectric current. As an example, we calculate the nonlinear Nernst and Hall current in the loop-current model for cuprate superconductors, and demonstrate their unique behaviour and capability of indicating $\mathcal{TI}$-invariance.