On the origin of asymmetric fission of actinides
Abstract
Nuclear fission of heavy (actinide) nuclei results predominantly in asymmetric mass-splits. Without quantum shells, which can give extra binding energy to these mass-asymmetric shapes, the nuclei would fission symmetrically. The strongest shell effects are in spherical nuclei, so naturally the spherical "doubly-magic" 132Sn nucleus (Z=50 protons), was expected to play a major role. However, a systematic study of fission has shown that the heavy fragments are distributed around Z=52 to 56, indicating that 132Sn is not the only driver. Reconciling the strong spherical shell effects at Z=50 with the different Z values of fission fragments observed in nature has been a longstanding puzzle. Here, we show that the final mass asymmetry of the fragments is also determined by the extra stability of octupole (pear-shaped) deformations which have been recently confirmed experimentally around 144Ba (Z=56), one of very few nuclei with shell-stabilized octupole deformation. Using a modern quantum many-body model of superfluid fission dynamics, we found that heavy fission fragments are produced predominantly with 52-56 protons, associated with significant octupole deformation acquired on the way to fission. These octupole shapes favouring asymmetric fission are induced by deformed shells at Z=52 and 56. In contrast, spherical "magic" nuclei are very resistant to octupole deformation, which hinders their production as fission fragments. These findings may explain surprising observations of asymmetric fission of lighter than lead nuclei.