Optically driven collective spin excitations and magnetization dynamics in the N\'eel-type skyrmion host GaV4S8

Abstract

GaV4S8 is a multiferroic semiconductor hosting magnetic cycloid (Cyc) and N\'eel-type skyrmion lattice (SkL) phases with a broad region of thermal and magnetic stability. Here, we use time-resolved magneto-optical Kerr spectroscopy and micro-magnetic simulations to demonstrate the coherent generation of collective spin excitations in the Cyc and SkL phases driven by an optically-induced modulation of uniaxial anisotropy. Our results shed light on spin-dynamics in anisotropic materials hosting skyrmions and pave a new pathway for the optical control of their magnetic order.

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