A Single-Crystal Neutron Diffraction Study on Magnetic Structure of CsCo2Se2

Abstract

The magnetic structure of CsCo2Se2 was investigated using single-crystal neutron diffraction technique. An antiferromagnetic transition with the propagation vector (0,0,1) was observed at TN = 78 K. The Co magnetic moment 0.772(6) μB at 10 K pointing in the basal plane couples ferromagnetically in the plane which stacks antiferromagnetically along the c direction. Tuning and suppressing the interplane antiferromagnetic interaction may be crucial to induce the material to a superconducting state.

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