Site Specific Knight Shift Measurements of the Dilute Kondo lattice System Ce1-xLaxCoIn5

Abstract

115In Nuclear magnetic resonance data are presented for a series of Ce1-xLaxCoIn5 crystals with different La dilutions, x. Multiple In(1) sites associated with different numbers of nearest-neighbor cerium atoms exhibit different Knight shifts and spin lattice relaxation rates. Analysis of the temperature dependence of these sites reveals both an evolution of the heavy electron coherence as a function of dilution, as well as spatial inhomogeneity associated with a complete suppression of antiferromagnetic fluctuations in the vicinity of the La sites. Quantum critical fluctuations persist within disconnected Ce clusters with dilution levels up to 75%, despite the fact that specific heat shows Fermi liquid behavior in dilute samples.

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