Signatures of quantized coupling between quantum emitters and localized surface plasmons

Abstract

Confining light to scales beyond the diffraction limit, quantum plasmonics supplies an ideal platform to explore strong light-matter couplings. The light-induced localized surface plasmons (LSPs) on the metal-dielectric interface acting as a quantum bus have wide potential in quantum information processing; however, the loss nature of light in the metal hinders their application. Here we propose a mechanism to make the reversible energy exchange and the multipartite quantum correlation of a collective of quantum emitters (QEs) mediated by the LSPs persistent. Via investigating the quantized interaction between the QEs and the LSPs supported by a spherical metal nanoparticle, we find that the diverse signatures of the quantized QE-LSP coupling in the steady state, including the complete decay, population trapping, and persistent oscillation, are essentially determined by the different number of bound states formed in the energy spectrum of the QE-LSP system. Enriching our understanding on the light-matter interactions in a lossy medium, our result is instructive in the design of quantum devices using plasmonic nanostructures.