Towards exciton-polaritons in MoS$_2$ nanotubes

Abstract

We measure low-temperature micro-photoluminescence spectra along a MoS$_2$ nanotube, which exhibit the peaks of the optical whispering gallery modes below the exciton resonance. The variation of the position and intensity of these peaks is used to quantify the change of the nanotube geometry. The width of the peaks is shown to be determined by the fluctuations of the nanotube wall thickness and propagation of the detected optical modes along the nanotube. We analyse the dependence of the energies of the optical modes on the wave vector along the nanotube axis and demonstrate the potential of the high-quality nanotubes for realization of the strong coupling between exciton and optical modes with the Rabi splitting reaching 400 meV. We show how the formation of exciton-polaritons in such structures will be manifested in the micro-photoluminescence spectra.