Long-term memory and delayed shear localisation in soft glassy materials

Abstract

We study theoretically the dynamics of soft glassy materials during the process of stress relaxation following the rapid imposition of a shear strain. By detailed numerical simulations of a mesoscopic soft glassy rheology model and three different simplified continuum fluidity models, we show that a dramatic shear localisation instability arises, in which the strain field suddenly becomes heterogeneous within the sample, accompanied by a precipitous drop in the stress. Remarkably, this instability can arise at extremely long delay times after the strain was applied, due to the long-term memory inherent to glassy systems. The finding that a catastrophic mechanical instability can arise long after any deformation could have far reaching consequences for material processing and performance, and potentially also for delayed geophysical phenomena.