Universal relationship between low-energy antiferromagnetic fluctuations and superconductivity in BaFe2(As1-xPx)2

Abstract

To identify the key parameter for optimal superconductivity in iron pnictides, we measured the 31P-NMR relaxation rate on BaFe2(As1-xPx)2 (x = 0.22 and 0.28) under pressure and compared the effects of chemical substitution and physical pressure. For x = 0.22, structural and antiferromagnetic (AFM) transition temperatures both show minimal changes with pressure up to 2.4~GPa, whereas the superconducting transition temperature T c increases to twice its former value. In contrast, for x=0.28 near the AFM quantum critical point (QCP), the structural phase transition is quickly suppressed by pressure and T c reaches a maximum. The analysis of the temperature-dependent nuclear relaxation rate indicates that these contrasting behaviors can be quantitatively explained by a single curve of the T c dome as a function of Weiss temperature θ, which measures the distance to the QCP. Moreover, the T c-θ curve under pressure precisely coincides with that with chemical substitution, which is indicative of the existence of a universal relationship between low-energy AFM fluctuations and superconductivity on BaFe2(As1-xPx)2.

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