Fragmented monopole crystal, dimer entropy and Coulomb interactions in Dy2Ir2O7
Abstract
Neutron scattering, specific heat and magnetisation measurements on both powders and single crystals reveal that Dy2Ir2O7 realizes the fragmented monopole crystal state in which antiferromagnetic order and a Coulomb phase spin liquid co-inhabit. The measured residual entropy is that of a hard core dimer liquid, as predicted. Inclusion of Coulomb interactions allows for a quantitative description of both the thermodynamic data and the magnetisation dynamics, with the energy scale given by deconfined defects in the emergent ionic crystal. Our data reveal low energy excitations, as well as a large distribution of energy barriers down to low temperatures, while the magnetic response to an applied field suggests that domain wall pinning is important; results that call for further theoretical modelling.