Time-reversal invariant and fully gapped unconventional superconducting state in the bulk of the topological Nb0.25Bi2Se3

Abstract

Recently, the niobium (Nb)-doped topological insulator Bi2Se3, in which the finite magnetic moments of the Nb atoms are intercalated in the van der Waals gap between the Bi2Se3 layers, has been shown to exhibit both superconductivity with Tc = 3 K and topological surface states. Here we report on muon spin rotation experiments probing the temperature-dependent of effective magnetic penetration depth Lambdaeff(T) in the layered topological superconductor candidate Nb0.25Bi2Se3. The exponential temperature dependence of lambda(eff)(-2)(T) at low temperatures suggests a fully gapped superconducting state in the bulk with the superconducting transition temperature Tc = 2.9 K and the gap to Tc ratio 2Delta/kBTc = 3.95(19). We also revealed that the ratio Tc/lambda(eff)(-2) is comparable to those of unconventional superconductors, which hints at an unconventional pairing mechanism. Furthermore, time reversal symmetry breaking was excluded in the superconducting state with sensitive zero-field muSR experiments. We hope the present results will stimulate theoretical investigations to obtain a microscopic understanding of the relation between superconductivity and the topologically non-trivial electronic structure of Nb0.25Bi2Se3.

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