Magnetic order of Dy3+ and Fe3+ moments in antiferromagnetic DyFeO3 probed by spin Hall magnetoresistance and spin Seebeck effect

Abstract

We report on spin Hall magnetoresistance (SMR) and spin Seebeck effect (SSE) in single crystal of the rare-earth antiferromagnet DyFeO3 with a thin Pt film contact. The angular shape and symmetry of the SMR at elevated temperatures reflect the antiferromagnetic order of the Fe3+ moments as governed by the Zeeman energy, the magnetocrystalline anisotropy and the Dzyaloshinskii-Moriya interaction. We interpret the observed linear dependence of the signal on the magnetic field strength as evidence for field-induced order of the Dy3+ moments up to room temperature. At and below the Morin temperature of 50\,K, the SMR monitors the spin-reorientation phase transition of Fe3+ spins. Below 23\,K, additional features emerge that persist below 4\,K, the ordering temperature of the Dy3+ magnetic sublattice. We conclude that the combination of SMR and SSE is a simple and efficient tool to study spin reorientation phase transitions and sublattice magnetizations.

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