Analyzing the Rydberg-based omg architecture for 171Yb nuclear spins

Abstract

Neutral alkaline earth(-like) atoms have recently been employed in atomic arrays with individual readout, control, and high-fidelity Rydberg-mediated entanglement. This emerging platform offers a wide range of new quantum science applications that leverage the unique properties of such atoms: ultra-narrow optical "clock" transitions and isolated nuclear spins. Specifically, these properties offer an optical qubit ("o") as well as ground ("g") and metastable ("m") nuclear spin qubits, all within a single atom. We consider experimentally realistic control of this "omg" architecture and its coupling to Rydberg states for entanglement generation, focusing specifically on ytterbium-171 (171Yb) with nuclear spin I = 1/2. We analyze the S-series Rydberg states of 171Yb, described by the three spin-1/2 constituents (two electrons and the nucleus). We confirm that the F = 3/2 manifold -- a unique spin configuration -- is well suited for entangling nuclear spin qubits. Further, we analyze the F = 1/2 series -- described by two overlapping spin configurations -- using a multichannel quantum defect theory. We study the multilevel dynamics of the nuclear spin states when driving the clock or Rydberg transition with Rabi frequency c = 2 π × 200 kHz or R = 2 π × 6 MHz, respectively, finding that a modest magnetic field (≈200\,G) and feasible laser polarization intensity purity (0.99) are sufficient for gate fidelities exceeding 0.99.

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