Higgs-Leggett mechanism for the elusive 6e superconductivity observed in Kagome vanadium-based superconductors

Abstract

A recent Little-Parks experiment on Kagome-structured superconductor CsV_3Sb_5 demonstrated remarkable resistance oscillations with period \phi0/3=hc/6e. Here, we perform analysis based on a theory involving three 2e superconductivity (SC) order parameters associated with the three reciprocal lattice vectors which connect M points of the hexagonal Brillouin zone. In a ring geometry we unveil that, as a series of metastable states, phase of one SC order parameter winds 2\pi more or less than the other two ones around the ring, which yields local free energy minima at integer multiples of \phi0/3. Intriguingly, the ground-state degeneracy associated with a Z_2 chirality is crucial, and the Higgs-Leggett mechanism stabilizes domain walls (DW) between chiral domains. At low temperatures DW are expelled from the system resulting in free energy minima only at integer multiples of \phi_0. Our theory explains successfully the 6e SC observed in experiments, which opens a door for approaching rich physics of Kagome superconductors.