Sublinear drag regime at mesoscopic scales in viscoelastic materials

Abstract

Stressed soft materials commonly present viscoelastic signatures in the form of power-law or exponential decay. Understanding the origins of such rheologic behaviors is crucial to find proper technological applications. Using an elastic network model of macromolecules immersed in a viscous fluid, we numerically reproduce those characteristic viscoelastic relaxations and show how the microscopic interactions determine the rheologic response. We find that exponential relaxations are indeed the most common behavior. However, power laws may arise when drag forces between the macromolecules and the fluid are sublinear, which is related to micro-deformations of the macromolecules.