High Chern numbers in a perovskite-derived dice lattice (La$X$O$_3$)$_3$/(LaAlO$_3$)$_3$(111) with $X=$ Ti, Mn and Co

Abstract

The dice lattice, containing a stack of three triangular lattices, has been proposed to exhibit nontrivial flat bands with nonzero Chern numbers, but unlike the honeycomb lattice it is much less studied. By employing density-functional theory (DFT) calculations with an on-site Coulomb repulsion term, we explore systematically the electronic and topological properties of (La$X$O$_3$)$_3$/(LaAlO$_3$)$_3$(111) superlattices with $X=$ Ti, Mn and Co, where a LaAlO$_3$ trilayer spacer confines the La$X$O$_3$ (L$X$O) dice lattice. In the absence of spin-orbit coupling (SOC) with symmetry constrained to P3, the ferromagnetic (FM) phase of the L$X$O(111) trilayers exhibits a distinct spin-polarized half-metallic state with multiple Dirac crossings and coupled electron-hole pockets around the Fermi energy. Symmetry lowering induces a significant rearrangement of bands and triggers a metal-to-insulator transition. Inclusion of SOC leads to a substantial anomalous Hall conductivity (AHC) around the Fermi energy reaching values up to $\sim-3e^2/h$ for $X=$ Mn and Co in P3 symmetry and both in- and out-of-plane magnetization directions in the first case and along [001] in the latter. The dice lattice emerges as a promising playground to realise nontrivial topological phases with high Chern numbers.