Direct numerical analysis of dynamic facilitation in glass-forming liquids

Abstract

We propose a computational strategy to quantify the temperature evolution of the timescales and lengthscales over which dynamic facilitation affects the relaxation dynamics of glass-forming liquids at low temperatures, that requires no assumption about the nature of the dynamics. In two glass models, we find that dynamic facilitation depends strongly on temperature, leading to a subdiffusive spreading of relaxation events which we characterize using a temperature-dependent dynamic exponent. We also establish that this temperature evolution represents a major contribution to the increase of the structural relaxation time.