Dynamical renormalization of the magnetic excitation spectrum via high-momentum nonlinear magnonics

Abstract

Controlling macroscopic properties of quantum materials requires the ability to induce and manipulate excited states. The set of collective excitations of a solid is encoded in its dispersion relations. We find that the spectra of the low-momentum eigenmodes are renormalized by resonantly driving the high-momentum excitations. Our experimental data rule out laser-induced thermal processes as an origin of the renormalization. The photoinduced changes of the amplitudes and frequencies can be explained theoretically and numerically with a resonant light-scattering mechanism that couples high- and low-momentum eigenmodes in the dispersion relation across momentum space. While we demonstrate the renormalization of the magnetic spectrum in a quantum material, our experimental approach can be further generalized to lattice modes in semiconductors.