A global study of α-clusters decay in heavy and superheavy nuclei with half-life and preformation factor
Abstract
A detailed study of α-clusters decay is exhibited by incorporating crucial microscopic nuclear structure information into the estimations of half-life and preformation factor. For the first time, using the k-cross validation approach, two semi-empirical formulas for (i) α-decay half-life and (ii) α-particle preformation factor, are picked out and subsequently modified by including shell, odd-nucleon blocking, and asymmetry effects along with the usual dependence on α-decay energy (Qα) and angular momentum of α-particle. Both the formulas are fitted for the two different regions separated by neutron number N=126, as from the experimental systematics the role of N=126 shell closure is found decisive in determining the trends of Qα, α-decay half-life, and α-particle preformation factor. It is found that the inclusion of the above-mentioned degrees of freedom significantly reduces the errors in the estimations when compared with several other similar modified/refitted semi-empirical relations indicating the robustness of the proposed formulas. The predictions of α-decay half-life throughout the periodic chart have been made including the unknown territory, future probable decay chain of self-conjugate nucleus 112Ba terminated on 100Sn, decay chain of 208Pa through new isotope 204Ac as well as decay chains of awaiting superheavy nuclei 298Og and 299120.
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