Field Dispersion and Strong Coupling of Nuclear-Electron Spin Excitation in MnCO3

Abstract

Hybridized nuclear and electron spin excitation in a MnCO3 crystal, a weakly-anisotropic antiferromagnet, has been investigated. In this material, the hyperfine interaction is strong enough to form a nuclear spin wave. We measure the microwave absorption by a bulk MnCO3 and observe the dispersion representing strong frequency repulsion between electron and nuclear modes due to their hybridization, the signature of nuclear spin wave. Additionally, we observe that the nuclear spin resonance enters a nonlinear regime above a certain excitation power, attributed to the excitation of finite wavenumber nuclear spin waves.

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